/
Article

Coherent Raman spectroscopy

MAY 01, 1977
Once exotic and time‐consuming, wave‐mixing spectroscopy has burgeoned into a set of techniques that can handle systems—flames, plasmas, luminescent crystals—inaccessible to conventional methods.
Marc D. Levenson

In 1928 Chandrasekhara Raman reported a process in which a material would simultaneously absorb one photon and emit another. The energies of the two photons differed by an amount corresponding to the energy difference between two quantum‐mechanical levels of the medium. Raman scattering, as the phenomenon came to be known, provided a tool for the spectroscopic investigation of energy levels not accessible by the usual absorption and emission techniques. For the first thirty‐five years Raman scattering was a laborious and exotic technique, important more for the quantum‐mechanical principles it illustrated than for its practical applications.

This article is only available in PDF format

References

  1. 1. M. C. Tobin, Laser Raman Spectroscopy, Wiley, New York (1971);
    T. R. Gilson, P. J. Hedra, Laser Raman Spectroscopy, Wiley, New York (1970).

  2. 2. C. Flytzanis, in Quantum Electronics, volume 1A (H. Rabin, C. Tang, eds.) Academic, New York (1975);
    C. Flytzanis, N. Bloembergen, in Progress in Quantum Electronics (J. H. Sanders, S. Stenholm, eds.) volume 4, part 3, Pergamon, New York (1976).

  3. 3. P. D. Maker, R. W. Terhune, Phys. Rev. A 137, 801 (1965).https://doi.org/PRVAAH

  4. 4. R. F. Begley, A. B. Harvey, R. L. Byer, Appl. Phys. Lett. 25, 387 (1975).https://doi.org/APPLAB

  5. 5. D. Heiman, R. W. Hellwarth, M. D. Levenson, G. Martin, Phys. Rev. Lett. 36, 189 (1976).https://doi.org/PRLTAO

  6. 6. I. Chabay, G. K. Klauminger, B. S. Hudson, Appl. Phys. Lett. 28, 27 (1975).https://doi.org/APPLAB

  7. 7. J. J. Song, G. L. Eesley, M. D. Levenson, Appl. Phys. Lett. 29, 567 (1976).https://doi.org/APPLAB

  8. 8. W. M. Tolles, J. W. Nibler, J. R. McDonald, A. G. Harvey, Appl. Spectroscopy 31, 96 (1977).https://doi.org/APSPA4

  9. 9. A. B. Harvey, J. R. McDonald, W. M. Tolles, in Progress in Analytical Chemistry, Plenum, New York (1977).

  10. 10. W. Kaiser, A. Laubareau, in Tunable Lasers and Applications (A. Mooradian, I. T. Jaeger, P. Stoketh, eds.), volume 3, Springer, New York (1976), page 207.

  11. 11. P. R. Regnier, in Laser Raman Gas Diagnostics, (M. Lapp, C. M. Penney, eds.) Plenum, New York (1974).

  12. 12. M. D. Levenson, N. Bloembergen, Phys. Rev. B 10, 4447 (1974).https://doi.org/PLRBAQ

  13. 13. P. Yaney, J. Raman Spectroscopy 5 (to be published).

  14. 14. H. Lotem, R. T. LynchJr, N. Bloembergen, Phys. Rev. A 14, 1748 (1976).https://doi.org/PLRAAN

  15. 15. W. T. Jones, B. P. Stoicheff, Phys. Rev. Lett. 13, 657 (1964).https://doi.org/PRLTAO

  16. 16. S. D. Kramer, N. Bloembergen, Phys. Rev. B 14, 4654 (1976).https://doi.org/PLRBAQ

  17. 17. T. Yajima, Opt. Comm. 14, 378 (1975).https://doi.org/OPCOB8

More about the authors

Marc D. Levenson, University of Southern California, Los Angeles.

Related content
/
Article
The thermodynamic and quantum mechanical properties of topological insulators provide a path toward scalable energy storage in information-based batteries.
/
Article
At the end of the turbulent 1960s, the postwar funding boom in US physics came to a crashing halt. The lessons learned then may be helpful to today’s physicists.
/
Article
Interviews with 22 successful early-career physical scientists and engineers reveal that networking has been one of the most critical ways to nurture their careers.
/
Article
Myriad solutions emerge in the stressful process of balancing professional ambition and personal happiness.
This Content Appeared In
pt-cover_1977_05.jpeg

Volume 30, Number 5

Get PT newsletters in your inbox

pt_newsletter_card_blue.png
PT The Week in Physics

A collection of PT's content from the previous week delivered every Monday.

pt_newsletter_card_darkblue.png
PT New Issue Alert

Be notified about the new issue with links to highlights and the full TOC.

pt_newsletter_card_pink.png
PT Webinars & White Papers

The latest webinars, white papers and other informational resources.

By signing up you agree to allow AIP to send you email newsletters. You further agree to our privacy policy and terms of service.