Nanoscale view of colossal magnetoresistance
DOI: 10.1063/PT.4.0801

Colossal magnetoresistance is aptly named. By subjecting a piece of appropriately doped manganite to a strong magnetic field and a moderately low temperature, one can raise its electrical conductivity by 10 000%. Despite its prodigious magnitude, CMR has not led to any commercial devices since its discovery 15 years ago. Still, it continues to fascinate physicists. At its most basic level, CMR arises as a paramagnetic insulating phase yields to a ferromagnetic conducting phase. But evidence suggests that a third, charge-ordered antiferromagnetic phase could play a role too. To elucidate the issue, Jing Tao of Brookhaven National Laboratory and her collaborators developed a new experimental technique. Called scanning electron nanoscale diffraction (SEND), their technique combines electron diffraction’s ability to reveal the presence of ordered structures with scanning microscopy’s ability to reveal those structures’ real-space distribution. The patches in the figure correspond to charge-ordered regions. As the temperature approaches the 253-K CMR transition, the volume occupied by the charge-ordered phase increases. Simulations by Elbio Dagotto of Oak Ridge National Laboratory and his collaborators suggest an explanation: The charge-ordered phase vies with the ferromagnetic phase to become the predominant phase below the transition temperature. Although it loses the battle, the charge-ordered phase nevertheless delays and thereby intensifies the onset of CMR. (J. Tao et al., Phys. Rev. Lett. 103, 097202, 2009.